Is the main service 200 or 400 amps? Assuming you have 400 amp. service I recommend you replace your main panelboard with a 400amp MCB panelboard that is equipped with 1-200amp circuit breaker and 2-100amp circuit breakers. You can use the circuit breakers to feed whatever building you want...
To peterp: You chose 90A fuse or C.B. for secondary, according to NEC table 450-3(b) the secondary protection should be 250% of 54.13A = 135.3A, why not use 125, 110, 100 or 90A fuse or C.B.?