The problem I see here is that none of 14 geometrical tolerance characteristics in ASME Y14.5 is able to define tolerance zone that could grab your intent directly.
I would suggest using perpendicularity tolerance between both axes.
Assign one cylindrical feature as a datum feature A by attaching datum feature symbol to the diameter of this datum cylinder and then attach perpendicularity feature control frame to the diameter of second cylinder.
|perp|dia.X.X|A|
Knowing the length of the axis that is toleranced and allowable angular deviation, you could calculate maximum value of diameter of above perpendicularity tolerance zone. That is why I said you are not able to do it directly.
Are your parts completly parallel, or just located to a datum plane? Your drawing looks like a rather complicated 3D projection. A 0[°] angle makes no sense in 2D.